Tuning Acid-Metal Synergy in m-Cresol Hydrodeoxygenation over Bifunctional Pt/Aluminosilicate Catalysts

James A. Hunns; Lee J. Durndell; Xingguang Zhang; Muxina Konarova; Adam F. Lee; Karen Wilson

doi:10.1021/acscatal.4c00402

Tuning Acid-Metal Synergy in m-Cresol Hydrodeoxygenation over Bifunctional Pt/Aluminosilicate Catalysts

James A. Hunns
, Lee J. Durndell
, Xingguang Zhang
, Muxina Konarova
, Adam F. Lee^*
, Karen Wilson^*

^*Corresponding author for this work

Aston University
University of Shanghai for Science and Technology
University of Queensland
Griffith University Queensland

Research output: Contribution to journal › Article › peer-review

Abstract

Strong synergy between proximate Bro̷nsted acid and metal sites over a Pt/amorphous silica-alumina (ASA) catalyst confers striking activity and selectivity enhancements for m-cresol hydrodeoxygenation to methylcyclohexane, a fuel additive and potential liquid organic hydrogen carrier for storing renewable energy.

Original language	English
Pages (from-to)	7052-7061
Number of pages	10
Journal	ACS Catalysis
Volume	14
Issue number	9
Early online date	22 Apr 2024
DOIs	https://doi.org/10.1021/acscatal.4c00402
Publication status	Published - 3 May 2024

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

ASJC Scopus subject areas

Catalysis
General Chemistry

Keywords

bifunctional
biofuel
biomass
catalysis
hydrodeoxygenation

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10.1021/acscatal.4c00402

Cite this

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title = "Tuning Acid-Metal Synergy in m-Cresol Hydrodeoxygenation over Bifunctional Pt/Aluminosilicate Catalysts",

abstract = "Strong synergy between proximate Bro̷nsted acid and metal sites over a Pt/amorphous silica-alumina (ASA) catalyst confers striking activity and selectivity enhancements for m-cresol hydrodeoxygenation to methylcyclohexane, a fuel additive and potential liquid organic hydrogen carrier for storing renewable energy.",

keywords = "bifunctional, biofuel, biomass, catalysis, hydrodeoxygenation",

author = "Hunns, \{James A.\} and Durndell, \{Lee J.\} and Xingguang Zhang and Muxina Konarova and Lee, \{Adam F.\} and Karen Wilson",

note = "Publisher Copyright: {\textcopyright} 2024 American Chemical Society.",

year = "2024",

month = may,

day = "3",

doi = "10.1021/acscatal.4c00402",

language = "English",

volume = "14",

pages = "7052--7061",

journal = "ACS Catalysis",

issn = "2155-5435",

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T1 - Tuning Acid-Metal Synergy in m-Cresol Hydrodeoxygenation over Bifunctional Pt/Aluminosilicate Catalysts

AU - Hunns, James A.

AU - Durndell, Lee J.

AU - Zhang, Xingguang

AU - Konarova, Muxina

AU - Lee, Adam F.

AU - Wilson, Karen

PY - 2024/5/3

Y1 - 2024/5/3

N2 - Strong synergy between proximate Bro̷nsted acid and metal sites over a Pt/amorphous silica-alumina (ASA) catalyst confers striking activity and selectivity enhancements for m-cresol hydrodeoxygenation to methylcyclohexane, a fuel additive and potential liquid organic hydrogen carrier for storing renewable energy.

AB - Strong synergy between proximate Bro̷nsted acid and metal sites over a Pt/amorphous silica-alumina (ASA) catalyst confers striking activity and selectivity enhancements for m-cresol hydrodeoxygenation to methylcyclohexane, a fuel additive and potential liquid organic hydrogen carrier for storing renewable energy.

KW - bifunctional

KW - biofuel

KW - biomass

KW - catalysis

KW - hydrodeoxygenation

UR - https://www.scopus.com/pages/publications/85191197735

U2 - 10.1021/acscatal.4c00402

DO - 10.1021/acscatal.4c00402

M3 - Article

AN - SCOPUS:85191197735

SN - 2155-5435

VL - 14

SP - 7052

EP - 7061

JO - ACS Catalysis

JF - ACS Catalysis

IS - 9

ER -

Tuning Acid-Metal Synergy in m-Cresol Hydrodeoxygenation over Bifunctional Pt/Aluminosilicate Catalysts

Abstract

UN SDGs

ASJC Scopus subject areas

Keywords

Access to Document

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